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다차원 탄소재료 연구단
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Redox- and light-switchable N-heterocyclic carbenes: A "soup-to-nuts" course on contemporary structure-activity relationships

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Title
Redox- and light-switchable N-heterocyclic carbenes: A "soup-to-nuts" course on contemporary structure-activity relationships
Author(s)
Yeonkyeong Ryu; Guillermo Ahumada; Bielawski C.W.
Publication Date
2019-04
Journal
CHEMICAL COMMUNICATIONS, v.55, no.31, pp.4451 - 4466
Publisher
ROYAL SOC CHEMISTRY
Abstract
Switchable catalysts respond to various types of stimuli in a manner that results in distinct structural or electronic changes. When each state exhibits a different activity, selectivity, or solubility, the corresponding catalyst may be used to control chemical reactions in a temporally- or spatially-resolved fashion. N-Heterocyclic carbenes (NHCs) are versatile scaffolds for building switchable catalysts and many examples that respond to changes in electrochemical potential or light have been introduced. Such types of switchable NHCs will be described in this Feature Article. The accompanying discussions include design considerations, characterization methodology, quantification of the underlying switching phenomena, and utility in catalytic applications. Challenges for the field as well as perspectives on potential opportunities for future development are also provided. © 2019 The Royal Society of Chemistry.
URI
https://pr.ibs.re.kr/handle/8788114/5861
ISSN
1359-7345
Appears in Collections:
Center for Multidimensional Carbon Materials(다차원 탄소재료 연구단) > Journal Papers (저널논문)
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