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Stereoelectronically-induced allosteric binding: shape complementarity promotes positive cooperativity in fullerene/buckybowl complexes

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Title
Stereoelectronically-induced allosteric binding: shape complementarity promotes positive cooperativity in fullerene/buckybowl complexes
Author(s)
Eric S. Larsen; Guillermo Ahumada; Prakash R. Sultane; Christopher W. Bielawski
Publication Date
2022-06
Journal
CHEMICAL COMMUNICATIONS, v.58, no.45, pp.6498 - 6501
Publisher
ROYAL SOC CHEMISTRY
Abstract
A novel 2 : 1 host-guest complex forms between 8-tert-butyl-6b(2)-azapenta-benzo[bc,ef,hi,kl,no]corannulene (1) and C-60 with positive cooperativity (alpha = 2.56) and high affinity (K-1 x K-2 = 2.8 x 10(6) M-2) at 25 degrees C. The C-60 undergoes increasing shape complementarity toward 1 throughout the binding process.
URI
https://pr.ibs.re.kr/handle/8788114/11939
DOI
10.1039/d2cc01908f
ISSN
1359-7345
Appears in Collections:
Center for Multidimensional Carbon Materials(다차원 탄소재료 연구단) > 1. Journal Papers (저널논문)
Center for Soft and Living Matter(첨단연성물질 연구단) > 1. Journal Papers (저널논문)
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