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Reversible disorder-order transitions in atomic crystal nucleation

DC Field Value Language
dc.contributor.authorSungho Jeon-
dc.contributor.authorTaeyeong Heo-
dc.contributor.authorSang-Yeon Hwang-
dc.contributor.authorJim Ciston-
dc.contributor.authorKaren C. Bustillo-
dc.contributor.authorBryan W. Reed-
dc.contributor.authorJimin Ham-
dc.contributor.authorNANOMAT-
dc.contributor.authorNANOMAT-
dc.contributor.authorJoowon Lim-
dc.contributor.authorKitaek Lim-
dc.contributor.authorNANOMAT-
dc.contributor.authorNANOMAT-
dc.contributor.authorRuth S. Bloom-
dc.contributor.authorSukjoon Hong-
dc.contributor.authorKwanpyo Kim-
dc.contributor.authorAlex Zettl-
dc.contributor.authorWoo Youn Kim-
dc.contributor.authorPeter Ercius-
dc.contributor.authorNANOMAT-
dc.contributor.authorWon Chul Lee-
dc.date.accessioned2021-04-13T04:50:09Z-
dc.date.accessioned2021-04-13T04:50:09Z-
dc.date.available2021-04-13T04:50:09Z-
dc.date.available2021-04-13T04:50:09Z-
dc.date.created2021-02-26-
dc.date.issued2021-01-
dc.identifier.issn0036-8075-
dc.identifier.urihttps://pr.ibs.re.kr/handle/8788114/9457-
dc.description.abstractNucleation in atomic crystallization remains poorly understood, despite advances in classical nucleation theory. The nucleation process has been described to involve a nonclassical mechanism that includes a spontaneous transition from disordered to crystalline states, but a detailed understanding of dynamics requires further investigation. In situ electron microscopy of heterogeneous nucleation of individual gold nanocrystals with millisecond temporal resolution shows that the early stage of atomic crystallization proceeds through dynamic structural fluctuations between disordered and crystalline states, rather than through a single irreversible transition. Our experimental and theoretical analyses support the idea that structural fluctuations originate from size-dependent thermodynamic stability of the two states in atomic dusters. These findings, based on dynamics in a real atomic system, reshape and improve our understanding of nucleation mechanisms in atomic crystallization.-
dc.description.uri1-
dc.language영어-
dc.publisherAMER ASSOC ADVANCEMENT SCIENCE-
dc.titleReversible disorder-order transitions in atomic crystal nucleation-
dc.typeArticle-
dc.type.rimsART-
dc.identifier.wosid000612983100041-
dc.identifier.scopusid2-s2.0-85100490924-
dc.identifier.rimsid74750-
dc.contributor.affiliatedAuthorNANOMAT-
dc.contributor.affiliatedAuthorNANOMAT-
dc.contributor.affiliatedAuthorNANOMAT-
dc.contributor.affiliatedAuthorNANOMAT-
dc.contributor.affiliatedAuthorKwanpyo Kim-
dc.contributor.affiliatedAuthorNANOMAT-
dc.identifier.doi10.1126/science.aaz7555-
dc.identifier.bibliographicCitationSCIENCE, v.371, no.6528, pp.498 - 503-
dc.citation.titleSCIENCE-
dc.citation.volume371-
dc.citation.number6528-
dc.citation.startPage498-
dc.citation.endPage503-
dc.description.journalClass1-
dc.description.isOpenAccessN-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.relation.journalWebOfScienceCategoryMultidisciplinary Sciences-
dc.subject.keywordPlusPARTICLE-SIZE-
dc.subject.keywordPlusELECTRON-
dc.subject.keywordPlusGROWTH-
dc.subject.keywordPlusTEM-
dc.subject.keywordPlusCRYSTALLIZATION-
dc.subject.keywordPlusNANOCRYSTALS-
dc.subject.keywordPlusMECHANISM-
dc.subject.keywordPlusCLUSTERS-
dc.subject.keywordPlusGOLD NANOPARTICLES-
Appears in Collections:
Center for Nanoparticle Research(나노입자 연구단) > 1. Journal Papers (저널논문)
Center for Nanomedicine (나노의학 연구단) > 1. Journal Papers (저널논문)
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