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Nanoscale Phenomena in Lithium-Ion Batteries

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Title
Nanoscale Phenomena in Lithium-Ion Batteries
Author(s)
Jung S.-K.; Hwang I.; Chang D.; Park K.-Y.; Kim S.J.; Seong W.M.; Eum D.; Park J.; Kim B.; Kim J.; Heo J.H.; Kisuk Kang
Publication Date
2020-07
Journal
Chemical Reviews, v.120, no.14, pp.6684 - 6737
Publisher
American Chemical Society
Abstract
The electrochemical properties and performances of lithium-ion batteries are primarily governed by their constituent electrode materials, whose intrinsic thermodynamic and kinetic properties are understood as the determining factor. As a part of complementing the intrinsic material properties, the strategy of nanosizing has been widely applied to electrodes to improve battery performance. It has been revealed that this not only improves the kinetics of the electrode materials but is also capable of regulating their thermodynamic properties, taking advantage of nanoscale phenomena regarding the changes in redox potential, solid-state solubility of the intercalation compounds, and reaction paths. In addition, the nanosizing of materials has recently enabled the discovery of new energy storage mechanisms, through which unexplored classes of electrodes could be introduced. Herein, we review the nanoscale phenomena discovered or exploited in lithium-ion battery chemistry thus far and discuss their potential implications, providing opportunities to further unveil uncharted electrode materials and chemistries. Finally, we discuss the limitations of the nanoscale phenomena presently employed in battery applications and suggest strategies to overcome these limitations
URI
https://pr.ibs.re.kr/handle/8788114/8944
DOI
10.1021/acs.chemrev.9b00405
ISSN
0009-2665
Appears in Collections:
Center for Nanoparticle Research(나노입자 연구단) > 1. Journal Papers (저널논문)
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