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Lee, Hyeong Jun
복잡계 이론물리 연구단
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Interplay between spin-orbit coupling and Van Hove singularity in the Hund's metallicity of Sr2RuO4

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Title
Interplay between spin-orbit coupling and Van Hove singularity in the Hund's metallicity of Sr2RuO4
Author(s)
Hyeong Jun Lee; Choong H. Kim; Ara Go
Subject
LAYERED PEROVSKITE, ; FERMI-SURFACE, ; SUPERCONDUCTIVITY, ; TRANSITION, ; STATES
Publication Date
2020-11
Journal
PHYSICAL REVIEW B, v.102, no.19, pp.195115
Publisher
AMER PHYSICAL SOC
Abstract
© 2020 American Physical Society. We investigate the roles of spin-orbit coupling and the Van Hove singularity in the dynamical properties of Sr2RuO4, which become prominent at zero and very low temperature, by means of density functional theory plus dynamical mean-field theory with an exact diagonalization solver. We examine the crossover between a Fermi liquid and a Hund's metal for a wide range of temperatures and Hund's coupling. In the absence of doping, we confirm that the Fermi liquid persists at zero temperature even with nonzero Hund's coupling. The freezing-moment mechanism suggests that thermal fluctuations lead to a suppression of the Fermi liquid phase and promote Hund's metallicity with incoherence. We show that the Van Hove singularity is an additional key ingredient to drive the suppression at very low temperature by observing a doping dependence of the freezing or long-lived paramagnetic moments. The role of spin-orbit coupling is marked by an amplified Van Vleck contribution of spin susceptibility, significantly promoting Hund's metallicity. Together with the known doping dependence of Hund's metallicity, the additional Van Hove singularity doping dependence found here may allow for the control of the Hund's metallicity of Sr2RuO4(t2g4) by a fine tuning of the doping or possibly even strain
URI
https://pr.ibs.re.kr/handle/8788114/7542
DOI
10.1103/PhysRevB.102.195115
ISSN
2469-9950
Appears in Collections:
Center for Theoretical Physics of Complex Systems(복잡계 이론물리 연구단) > 1. Journal Papers (저널논문)
Center for Correlated Electron Systems(강상관계 물질 연구단) > 1. Journal Papers (저널논문)
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