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나노입자 연구단
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Effect of N-doped carbon coatings on the durability of highly loaded platinum and alloy catalysts with different carbon supports for polymer electrolyte membrane fuel cells

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Title
Effect of N-doped carbon coatings on the durability of highly loaded platinum and alloy catalysts with different carbon supports for polymer electrolyte membrane fuel cells
Author(s)
Chi-Yeong Ahn; Wonchan Hwang; Hyunjoon Lee; Sungjun Kim; Ji Eun Park; Ok-Hee Kim; Min Her; Yong-Hun Cho; Yung-Eun Sung
Publication Date
2018-05
Journal
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, v.43, no.21, pp.10070 - 10081
Publisher
PERGAMON-ELSEVIER SCIENCE LTD
Abstract
An ideal oxygen reduction catalyst for use in fuel cells should exhibit both long-term durability and high activity. In this study, to increase the durability of highly loaded platinum- and platinum-nickel alloy catalysts possessing different types of carbon supports, a nitrogen-doped carbon shell was introduced on the catalyst surface through dopamine coating. As the catalyst surfaces were altered following shell formation, the ionomer contents of the catalyst inks were adjusted to optimise the three-phase boundary formation. Single cell tests were then conducted on these inks by applying them in a membrane electrolyte assembly. Furthermore, to confirm the durability of the catalysts under accelerated conditions, the operation was continued for 200 h at 70 C and at a relative humidity of 100%. Transmission electron microscopy and electrochemical analysis were conducted before and after the durability tests, and the observed phenomena were discussed for catalysts bearing different types of carbon supports. © 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
URI
https://pr.ibs.re.kr/handle/8788114/5569
ISSN
0360-3199
Appears in Collections:
Center for Nanoparticle Research(나노입자 연구단) > Journal Papers (저널논문)
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