Stepwise synthesis via mechanochemical reaction for multistate redox-active 2D Zinc(ii) coordination network

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Title
Stepwise synthesis via mechanochemical reaction for multistate redox-active 2D Zinc(ii) coordination network
Author(s)
Joo Yeon Ha; Deekamwong K.; Ohtsu H.; Kimoon Kim; Hashizume D.; Kawano M.
Publication Date
2018-09
Journal
CHEMISTRY LETTERS, v.47, no.9, pp.1184 - 1186
Publisher
CHEMICAL SOC JAPAN
Abstract
A multistate redox-active coordination network was prepared by stepwise synthesis via mechanochemical reaction to overcome the low solubility of ligands. Solid-state grinding between sparingly soluble ligands and metal ions lead to the formation of a soluble intermediate. A two-dimensional (2D) coordination network possessing open channels and iodinated pores was prepared by using the intermediate. The redox activity of the network, which was derived from ligands, was confirmed by electron spin resonance (ESR) spectroscopy and solid-state cyclic voltammetry. © 2018 The Chemical Society of Japan
URI
https://pr.ibs.re.kr/handle/8788114/4925
ISSN
0366-7022
Appears in Collections:
Center for Self-assembly and Complexity(복잡계 자기조립 연구단) > Journal Papers (저널논문)
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