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나노 구조 물리 연구단
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Thickness-dependent in-plane thermal conductivity of suspended MoS2 grown by chemical vapor deposition

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Title
Thickness-dependent in-plane thermal conductivity of suspended MoS2 grown by chemical vapor deposition
Author(s)
Jung Jun Bae; Hye Yun Jeong; Gang Hee Han; Jaesu Kim; Hyun Kim; Min Su Kim; Byoung Hee Moon; Seong Chu Lim; Young Hee Lee
Publication Date
2017-02
Journal
Nanoscale, v.9, no.7, pp.2541 - 2547
Publisher
ROYAL SOC CHEMISTRY
Abstract
The in-plane thermal conductivities of suspended monolayer, bilayer, and multilayer MoS2 films were measured in vacuum by using non-invasive Raman spectroscopy. The samples were prepared by chemical vapor deposition (CVD) and transferred onto preformed cavities on a Au-coated SiO2/Si substrate. The measured thermal conductivity (13.3 ± 1.4 W m−1 K−1) of the suspended monolayer MoS2 was below the previously reported value of 34.5 ± 4 W m−1 K−1. We demonstrate that this discrepancy arises from the experimental conditions that differ from vacuum conditions and small absorbance. The measured in-plane thermal conductivity of the suspended MoS2 films increased in proportion to the number of layers, reaching 43.4 ± 9.1 W m−1 K−1 for the multilayer MoS2, which explicitly follows the Fuchs-Sondheimer suppression function. The increase in the thermal conductivity with the number of MoS2 layers is explained by the reduced phonon boundary scattering. We also observe that the Fuchs-Sondheimer model works for the thickness-dependent thermal conductivity of MoS2 down to 10 nm in thickness at room temperature, yielding a phonon mean free path of 17 nm for bulk. © The Royal Society of Chemistry
URI
https://pr.ibs.re.kr/handle/8788114/3467
ISSN
2040-3364
Appears in Collections:
Center for Integrated Nanostructure Physics(나노구조물리 연구단) > Journal Papers (저널논문)
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