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나노 구조 물리 연구단
나노구조물리 연구단
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Flexible High-Performance Lead-Free Na0.47K0.47Li0.06NbO3 Microcube-Structure-Based Piezoelectric Energy Harvester

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Title
Flexible High-Performance Lead-Free Na0.47K0.47Li0.06NbO3 Microcube-Structure-Based Piezoelectric Energy Harvester
Author(s)
Gupta, MK; Sang-Woo Kim; Kumar, B
Publication Date
2016-01
Journal
ACS APPLIED MATERIALS & INTERFACES, v.8, no.3, pp.1766 - 1773
Publisher
AMER CHEMICAL SOC
Abstract
Lead-free piezoelectric nano- and microstructure-based generators have recently attracted much attention due to the continuous demand of self-powered body implantable devices. We report the fabrication of a high-performance flexible piezoelectric microgenerator based on lead-free inorganic piezoelectric Na0.47K0.47Li0.06NbO3 (NKLN) microcubes for the first time. The composite generator is fabricated using NKLN microcubes and polydimethylsiloxane (PDMS) polymer on a flexible substrate. The flexible device exhibits excellent performance with a large recordable piezoelectric output voltage of 48 V and output current density of 0.43 mu A/cm(2) under vertical compressive force of 2 kgf, for which an energy conversion efficiency of about 11% has been achieved. Piezoresponse and ferroelectric studies reveal that NKLN microcubes exhibited high piezoelectric charge coefficient (d(33)) as high as 460 pC/N and a well-defined hysteresis loops with remnant polarization and coercive field of 13.66 mu C/cm(2) and 19.45 kV/cm, respectively. The piezoelectric charge generation mechanism from NKLN microgenerator are discussed in the light of the high d33 and alignment of electric dipoles in polymer matrix and dielectric constant of NKLN microcubes. It has been demonstrated that the developed power generator has the potential to generate high electric output power under mechanical vibration for powering biomedical devices in the near future. © 2016 American Chemical Society
URI
https://pr.ibs.re.kr/handle/8788114/2560
ISSN
1944-8244
Appears in Collections:
Center for Integrated Nanostructure Physics(나노구조물리 연구단) > Journal Papers (저널논문)
Files in This Item:
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