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Unraveling the surface self-reconstruction of Fe-doped Ni-thiophosphate for efficient oxygen evolution reaction

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Title
Unraveling the surface self-reconstruction of Fe-doped Ni-thiophosphate for efficient oxygen evolution reaction
Author(s)
Kirubasankar, Balakrishnan; Won, Yo Seob; Soo Ho Choi; Kim, Jae Woo; Adofo, Laud Anim; Kim, Soo Min; Ki Kang Kim
Publication Date
2023-07
Journal
CHEMICAL COMMUNICATIONS, v.59, no.60, pp.9247 - 9250
Publisher
ROYAL SOC CHEMISTRY
Abstract
Surface self-reconstruction of oxygen evolution reaction (OER) electrocatalysts generally occurs during the electrochemical activation process. Herein, we study the surface self-reconstruction of a 2D layered Fe-doped Ni-thiophosphate (NixFe1-xPS3) nanosheet. The role of Fe in the surface self-reconstruction of NiPS3 during the OER is investigated by using an in situ Raman analysis. Formation of amorphous metal/non-metal oxide layers on the surface of NixFe1-xPS3 can efficiently act as the ultimate catalytic center for the OER. © The Royal Society of Chemistry 2023
URI
https://pr.ibs.re.kr/handle/8788114/13762
DOI
10.1039/d3cc01510f
ISSN
1359-7345
Appears in Collections:
Center for Integrated Nanostructure Physics(나노구조물리 연구단) > 1. Journal Papers (저널논문)
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