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Structure-sensitive epoxidation of dicyclopentadiene over TiO2 catalysts

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Title
Structure-sensitive epoxidation of dicyclopentadiene over TiO2 catalysts
Author(s)
Chung, Sang-Ho; G. Hwan Park; Schukkink, Niels; Hyoyoung Lee; Shiju, N. Raveendran
Publication Date
2023-01
Journal
Chemical Communications, v.59, no.6, pp.756 - 759
Publisher
Royal Society of Chemistry
Abstract
© Royal Society of Chemistry 2023. Epoxidation of dicyclopentadiene (DCPD) is studied on a series of TiO2 catalysts using hydrogen peroxide as an oxidant. DCPD derivatives have applications in several areas including polymer, pharmaceutical and pesticide products. The control of selectivity leading to the desired product is important for many of these applications. Using experimental and computational studies, we show that the surface crystalline phases of TiO2 play crucial roles not only in the formation of peroxo species but also in the selective epoxidation of two different C=C double bonds in DCPD.
URI
https://pr.ibs.re.kr/handle/8788114/12444
DOI
10.1039/d2cc05305e
ISSN
1359-7345
Appears in Collections:
Center for Integrated Nanostructure Physics(나노구조물리 연구단) > 1. Journal Papers (저널논문)
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