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Reversible ammonia uptake at room temperature in a robust and tunable metal-organic framework

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Title
Reversible ammonia uptake at room temperature in a robust and tunable metal-organic framework
Author(s)
Jaechul Lee; Younggyu Seo; Kang, Dong Won; Seungjae Park; Hyunyong Kim; Kim, Jaheon; Kimoon Kim; Hong, Chang Seop; Lim, Dae-Woon; Lee, Eunsung
Publication Date
2022-03
Journal
RSC ADVANCES, v.12, no.13, pp.7605 - 7611
Publisher
ROYAL SOC CHEMISTRY
Abstract
Ammonia is useful for the production of fertilizers and chemicals for modern technology, but its high toxicity and corrosiveness are harmful to the environment and human health. Here, we report the recyclable and tunable ammonia adsorption using a robust imidazolium-based MOF (JCM-1) that uptakes 5.7 mmol g(-1) of NH3 at 298 K reversibly without structural deformation. Furthermore, a simple substitution of NO3- with Cl- in a post-synthetic manner leads to an increase in the NH3 uptake capacity of JCM-1(Cl-) up to 7.2 mmol g(-1).
URI
https://pr.ibs.re.kr/handle/8788114/11579
DOI
10.1039/d2ra01270g
ISSN
2046-2069
Appears in Collections:
Center for Self-assembly and Complexity(복잡계 자기조립 연구단) > 1. Journal Papers (저널논문)
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