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Locally enhanced light–matter interaction of MoS2 monolayers at density-controllable nanogrooves of template-stripped Ag films

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Title
Locally enhanced light–matter interaction of MoS2 monolayers at density-controllable nanogrooves of template-stripped Ag films
Author(s)
Jung Ho Kim; Lee, Jubok; Sehwan Park; Seo, Changwon; Seok Joon Yun; Han, Gang Hee; Kim, Jeongyong; Young Hee Lee; Lee, Hyun Seok
Publication Date
2022-01
Journal
Current Applied Physics, v.33, pp.59 - 65
Publisher
Elsevier B.V.
Abstract
© 2021Transition metal dichalcogenide (TMD) monolayers, such as MoS2, possess a direct optical bandgap are useful for emerging ultrathin optoelectronics in the visible light range, whereas their thin thickness limits light absorption and emission properties. To address this drawback, one promising approach is to hybridize plasmonic nanostructures with monolayer TMDs to utilize local field enhancement effects owing to localized surface plasmon resonance (LSPR). Herein, we propose a strong enhancement of the local light–matter interaction in MoS2 monolayers on naturally generated nanoscale grooves. The nanogrooves are formed at grain boundaries (GBs) of template-stripped metal film substrates that are fabricated by mechanically stripping Ag films deposited on an ultra-flat Si substrate, wherein the nanogroove densities are systematically modulated by the Ag film thickness. We observe an effective photoluminescence enhancement factor of 758 and a Raman spectroscopy intensity enhancement of approximately 5 times in MoS2 on the subwavelength-scale nanogrooves, compared with that on grain planes, which is attributed to a strong local field enhancement of the LSPR effect. Moreover, this plasmonic enhancement effect is elucidated by dark-field scattering spectroscopy and optical simulations. Our results can facilitate the utilization of density-controllable plasmonic nanogrooves synthesized without nanopatterning techniques for plasmonic hybrids on 2D semiconductors.
URI
https://pr.ibs.re.kr/handle/8788114/10985
DOI
10.1016/j.cap.2021.11.002
ISSN
1567-1739
Appears in Collections:
Center for Integrated Nanostructure Physics(나노구조물리 연구단) > 1. Journal Papers (저널논문)
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