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Quartz-based flat-crystal resonant inelastic x-ray scattering spectrometer with sub-10 meV energy resolution

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Title
Quartz-based flat-crystal resonant inelastic x-ray scattering spectrometer with sub-10 meV energy resolution
Author(s)
Jungho Kim; D.Casa; Alman Said; Rich Krakora; Bum Jun Kim; Elina Kasman; Xianrong Huang; T. Gog
Publication Date
2018-01
Journal
SCIENTIFIC REPORTS, v.8, no.1, pp.1958
Publisher
NATURE PUBLISHING GROUP
Abstract
Continued improvement of the energy resolution of resonant inelastic x-ray scattering (RIXS) spectrometers is crucial for fulfilling the potential of this technique in the study of electron dynamics in materials of fundamental and technological importance. In particular, RIXS is the only alternative tool to inelastic neutron scattering capable of providing fully momentum resolved information on dynamic spin structures of magnetic materials, but is limited to systems whose magnetic excitation energy scales are comparable to the energy resolution. The state-of-the-art spherical diced crystal analyzer optics provides energy resolution as good as 25 meV but has already reached its theoretical limit. Here, we demonstrate a novel sub-10 meV RIXS spectrometer based on flat-crystal optics at the Ir-L3 absorption edge (11.215 keV) that achieves an analyzer energy resolution of 3.9 meV, very close to the theoretical value of 3.7 meV. In addition, the new spectrometer allows efficient polarization analysis without loss of energy resolution. The performance of the instrument is demonstrated using longitudinal acoustical and optical phonons in diamond, and magnon in Sr3Ir2O7. The novel sub-10 meV RIXS spectrometer thus provides a window into magnetic materials with small energy scales. © The Author(s) 2018
URI
https://pr.ibs.re.kr/handle/8788114/5302
DOI
10.1038/s41598-018-20396-z
ISSN
2045-2322
Appears in Collections:
Center for Artificial Low Dimensional Electronic Systems(원자제어 저차원 전자계 연구단) > 1. Journal Papers (저널논문)
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Sceintific Reports_김범준(공동)_Quartz-based flat-crystal resonant inelastic x-ray scattering spectrometer with sub-10 meV energy resolution.pdfDownload

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