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Directed C−H Activation and Tandem Cross-Coupling Reactions Using Palladium Nanocatalysts with Controlled Oxidation

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Title
Directed C−H Activation and Tandem Cross-Coupling Reactions Using Palladium Nanocatalysts with Controlled Oxidation
Author(s)
Kim K.; Jung Y.; Lee S.; Kim M.; Shin D.; Byun H.; Cho S.J.; Hyunjoon Song; Hyunwoo Kim
Subject
cross-coupling, ; C−H activation, ; heterogeneous catalysis, ; nanoparticles, ; palladium
Publication Date
2017-06
Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.56, no.24, pp.6952 - 6956
Publisher
WILEY-V C H VERLAG GMBH
Abstract
Controlled oxidation of palladium nanoparticles provided high-valent PdIV oxo-clusters which efficiently promote directed C−H halogenation reactions. In addition, palladium nanoparticles can undergo changes in oxidation states to provide both high-valent PdIV and low-valent Pd0 species within one system, and thus a tandem reaction of C−H halogenation and cross-coupling (C−N, C−C, and C−S bond formation) was successfully established. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinhei
URI
https://pr.ibs.re.kr/handle/8788114/3616
DOI
10.1002/anie.201700301
ISSN
1433-7851
Appears in Collections:
Center for Nanomaterials and Chemical Reactions(나노물질 및 화학반응 연구단) > 1. Journal Papers (저널논문)
Files in This Item:
Angew.Chem. Int.Ed. 2017, 56,6952 –6956.pdfDownload

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