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Metal ion (Ca2+, Mg2+, Zn2+) catalyzed synthesis of high-quality zeolite templated carbon

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Title
Metal ion (Ca2+, Mg2+, Zn2+) catalyzed synthesis of high-quality zeolite templated carbon
Author(s)
Guangwu Yang; Li, Liangbin; Liu, Hao; Cheng, Yuanzhuang; Chen, Yanli; Li, Xiyou
Publication Date
2022-05-01
Journal
Microporous and Mesoporous Materials, v.336
Publisher
Elsevier B.V.
Abstract
© 2022 Elsevier Inc.Three metal ions (Ca2+, Mg2+, and Zn2+) were found to be successful catalysts to produce high-quality zeolite templated carbon (ZTC), a periodic three-dimensional graphene-like carbon with ordered microporous structure. Their roles in high-quality ZTC formation were studied by characterizing chemical component, surface morphology, structure, and pore properties. Ca2+, Mg2+, and Zn2+ minimize or eliminate the blockage of channels by carbon deposits and non-selective thermal deposition on the external surface of the zeolite particles. The growth temperature was lowered to only 450 °C. Moreover, the formation mechanism of ordered ZTC structure was revealed for the first time.
URI
https://pr.ibs.re.kr/handle/8788114/11404
DOI
10.1016/j.micromeso.2022.111860
ISSN
1387-1811
Appears in Collections:
Center for Multidimensional Carbon Materials(다차원 탄소재료 연구단) > 1. Journal Papers (저널논문)
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