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IBS Publications RepositoryCenter for Catalytic Hydrocarbon Functionalizations(분자활성 촉매반응 연구단)1. Journal Papers (저널논문)
Reactivity of Morita-Baylis-Hillman Adducts in C-H Functionalization of (Hetero)aryl Nitrones: Access to Bridged Cycles and Carbazoles
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- Title
- Reactivity of Morita-Baylis-Hillman Adducts in C-H Functionalization of (Hetero)aryl Nitrones: Access to Bridged Cycles and Carbazoles
- Author(s)
- Ashok Kumar Pandey; Dahye Kang; Sang Hoon Han; Heeyoung Lee; Neeraj Kumar Mishra; Hyung Sik Kim; Young Hoon Jung; Sungwoo Hong; In Su Kim
- Publication Date
- 2018-08
- Journal
- ORGANIC LETTERS, v.20, no.15, pp.4632 - 4636
- Publisher
- AMER CHEMICAL SOC
- Abstract
- The rhodium(III)-catalyzed cross-coupling of (hetero)aryl nitrones with Morita-Baylis-Hillman (MBH) adducts is described. An allylated intermediate derived from aryl nitrones and MBH adducts allows the formation of bridged cyclic compounds via an exotype [3 + 2] cycloaddition. In sharp contrast, electron-rich indolinyl or aniline substrates were found to couple with MBH adducts to generate naphthalene or carbazole derivatives, respectively. © 2018 American Chemical Society
- ISSN
- 1523-7060
- Appears in Collections:
- Center for Catalytic Hydrocarbon Functionalizations(분자활성 촉매반응 연구단) > 1. Journal Papers (저널논문)
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