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구진영
원자제어 저차원 전자계 연구단
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Spectroscopic, electronic and computational properties of a mixed tetrachalcogenafulvalene and its charge transfer complex

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Title
Spectroscopic, electronic and computational properties of a mixed tetrachalcogenafulvalene and its charge transfer complex
Author(s)
Walwyn R.J.; Chan B.; Usov P.M.; Solomon M.B.; Duyker S.G.; Jiin Young Koo; Masaki Kawano; Turner P.; Kepert C.J.; D'Alessandro D.M.
Publication Date
2018-02
Journal
Journal of Materials Chemistry C, v.6, no.5, pp.1092 - 1104
Publisher
ROYAL SOC CHEMISTRY
Abstract
This paper reports additional properties of the electron donor molecule triselenathiafulvalene (TSTF) and its synthesis via a new route involving the precursor tetracarbomethoxytriselenathiafulvalene (TCMTSTF). The structural, electronic and computational properties of TSTF are fully profiled, and discussed in the context of the closely related archetypal electron donor molecule tetrathiafulvalene (TTF). TSTF was also incorporated into a charge transfer (CT) complex with the well-known electron acceptor 7,7,8,8-tetracyanoquinodimethane (TCNQ), to generate TSTF-TCNQ. In order to establish its position in the greater TXF-TCNQ series (where TXF = a tetrachalcogenafulvalene), spectral, electrochemical, magnetic, conductivity and computational studies were performed on TSTF and TSTF-TCNQ to extend what is known about the highly interesting and useful new donor molecule. © 2018 The Royal Society of Chemistry
URI
https://pr.ibs.re.kr/handle/8788114/4447
ISSN
2050-7526
Appears in Collections:
Center for Artificial Low Dimensional Electronic Systems(원자제어 저차원 전자계 연구단) > Journal Papers (저널논문)
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