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Improved solar cell performance of Cu2ZnSnS4 (CZTS) thin films prepared by sulfurizing stacked precursor thin films via SILAR method

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Title
Improved solar cell performance of Cu2ZnSnS4 (CZTS) thin films prepared by sulfurizing stacked precursor thin films via SILAR method
Author(s)
Suryawanshi M.P.; Seung Wook Shin; Ghorpade U.V.; Gurav K.V.; Hong C.W.; Patil P.S.; Moholkar A.V.; Kim J.H.
Publication Date
2016-06
Journal
JOURNAL OF ALLOYS AND COMPOUNDS, v.671, no., pp.509 - 516
Publisher
ELSEVIER SCIENCE SA
Abstract
This paper describes an approach to using the successive ionic adsorption and reaction (SILAR) method for the synthesis of Cu2ZnSnS4 (CZTS), a highly promising thin film absorber material. This approach involves the preparation of stacked precursor thin films of Cu2SnS3 and ZnS by using the SILAR method with different stacking orders, such as Mo/Cu2SnS3/ZnS (CZTS-A) and Mo/ZnS/Cu2SnS3 (CZTS-B). These stacked precursor films were sulfurized at 575°C for 1 h in a H2S (5%) + N2 (95%) atmosphere. The characteristics of the CZTS thin films prepared using stacked sulfide precursors are strongly dependent on the stacking orders in the precursor thin films. The influence of different precursor stacking orders on the structural, compositional, morphological and optical properties as well as the photoelectrochemical (PEC) performance of the CZTS thin films were studied. The best PEC performance of 1.81% was obtained with a maximum Jsc of 11.68 mA/cm2, Voc of 0.42 V and FF of 0.37 for the CZTS thin films based on the stacking order of Mo/ZnS/Cu2SnS3. © 2016 Elsevier B.V. All rights reserved.
URI
https://pr.ibs.re.kr/handle/8788114/3152
ISSN
0925-8388
Appears in Collections:
Center for Nanomaterials and Chemical Reactions(나노물질 및 화학반응 연구단) > Journal Papers (저널논문)
Files in This Item:
Journal of Alloys and Compounds 671 (2016) 509e516.pdfDownload

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