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Two-Dimensionally Grown Single-Crystal Silicon Nanosheets with Tunable Visible-light Emissions

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Title
Two-Dimensionally Grown Single-Crystal Silicon Nanosheets with Tunable Visible-light Emissions
Author(s)
Sung Wook Kim; Jaejun Lee; Ji Ho Sung; Dong-jae Seo; Ilsoo Kim; Moon-Ho Jo; Byoung Wook Kwon; Won Kook Choi; Heon-Jin Choi
Subject
Si nanosheets . 2D growth . thickness-dependent photoluminescence . tunable emission
Publication Date
2014-07
Journal
ACS NANO, v.8, no.7, pp.6556 - 6562
Publisher
AMER CHEMICAL SOC
Abstract
Since the discovery of graphene, growth of twodimensional (2D) nanomaterials has greatly attracted attention. However, spontaneous growth of atomic two-dimensional (2D) materials is limitedly permitted for several layered-structure crystals, such as graphene, MoS2, and h-BN, and otherwise it is notoriously difficult. Here we report the gas-phase 2D growth of silicon (Si), that is cubic in symmetry, via dendritic growth and an interdendritic filling mechanism and to form Si nanosheets (SiNSs) of 1 to 13 nm in thickness. Thin SiNSs show strong thickness-dependent photoluminescence in visible range including red, green, and blue (RGB) emissions with the associated band gap energies ranging from 1.6 to 3.2 eV; these emission energies were greater than those from Si quantum dots (SiQDs) of the similar sizes. We also demonstrated that electrically driven white, as well as blue, emission in a conventional organic light-emitting diode (OLED) geometry with the SiNS assembly as the active emitting layers. Tunable light emissions in visible range in our observations suggest practical implications for novel 2D Si nanophotonics.
URI
https://pr.ibs.re.kr/handle/8788114/1485
DOI
10.1021/nn501683f
ISSN
1936-0851
Appears in Collections:
Center for Artificial Low Dimensional Electronic Systems(원자제어 저차원 전자계 연구단) > 1. Journal Papers (저널논문)
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12._ACSNano_8(7)_Two-Dimensionally_Grown_Single-Crystal_Silicon_Nanosheets_.pdfDownload

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