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나노물질및화학반응연구단
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Selective p-xylene production from biomass-derived dimethylfuran and ethylene over zeolite beta nanosponge catalysts

DC Field Value Language
dc.contributor.authorKim T.-W.-
dc.contributor.authorKim S.-Y.-
dc.contributor.authorJeong-Chul Kim-
dc.contributor.authorYoungjin Kim-
dc.contributor.authorRyong Ryoo-
dc.contributor.authorKim C.-U.-
dc.date.available2016-07-05T06:36:14Z-
dc.date.created2016-01-22-
dc.date.issued2016-05-
dc.identifier.issn0926-3373-
dc.identifier.urihttps://pr.ibs.re.kr/handle/8788114/2604-
dc.description.abstractp-Xylene can be synthesized via a renewable route from biomass-derived 2,5-dimethylfuran (DMF) and ethylene with zeolite catalysts. Here, we propose mesoporous beta zeolite with a nanosponge-like morphology (NSP-BEA) as a highly efficient catalyst for the cycloaddition of DMF with ethylene. The NSP-BEA zeolite was synthesized through a hydrothermal synthesis route using multi-ammonium surfactants as a meso-micro dual structure-directing agent. From structural analyses and measurements of the surface acidity, the NSP-BEA was found to be composed of ultrathin zeolitic nanocrystals with intercrystalline mesopores (~4.5. nm). It also possessed a large number of Brønsted acid sites on its external surfaces and in its internal micropores. This NSP-BEA catalyst exhibited high catalytic performance upon a cycloaddition of DMF with ethylene as compared to the commercial beta zeolite, alumina, and silica-alumina catalysts reported previously. © 2015 Elsevier B.V-
dc.description.uri1-
dc.language영어-
dc.publisherELSEVIER SCIENCE BV-
dc.subjectBeta zeolite-
dc.subjectCycloaddition-
dc.subjectDimethylfuran-
dc.subjectMesoporous zeolite-
dc.subjectP-Xylene-
dc.titleSelective p-xylene production from biomass-derived dimethylfuran and ethylene over zeolite beta nanosponge catalysts-
dc.typeArticle-
dc.type.rimsART-
dc.identifier.wosid000369452000010-
dc.identifier.scopusid2-s2.0-84949871178-
dc.identifier.rimsid22141ko
dc.date.tcdate2018-10-01-
dc.contributor.affiliatedAuthorJeong-Chul Kim-
dc.contributor.affiliatedAuthorYoungjin Kim-
dc.contributor.affiliatedAuthorRyong Ryoo-
dc.identifier.doi10.1016/j.apcatb.2015.11.046-
dc.identifier.bibliographicCitationAPPLIED CATALYSIS B-ENVIRONMENTAL, v.185, pp.100 - 109-
dc.citation.titleAPPLIED CATALYSIS B-ENVIRONMENTAL-
dc.citation.volume185-
dc.citation.startPage100-
dc.citation.endPage109-
dc.date.scptcdate2018-10-01-
dc.description.wostc25-
dc.description.scptc25-
dc.description.journalClass1-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.subject.keywordAuthorBeta zeolite-
dc.subject.keywordAuthorCycloaddition-
dc.subject.keywordAuthorDimethylfuran-
dc.subject.keywordAuthorMesoporous zeolite-
dc.subject.keywordAuthorP-Xylene-
Appears in Collections:
Center for Nanomaterials and Chemical Reactions(나노물질 및 화학반응 연구단) > 1. Journal Papers (저널논문)
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