Resolving Multiple Molecular Orbitals Using Two-Dimensional High-Harmonic Spectroscopy
DC Field | Value | Language |
---|---|---|
dc.contributor.author | Hyeok Yun | - |
dc.contributor.author | Kyung-Min Lee | - |
dc.contributor.author | Jae Hee Sung | - |
dc.contributor.author | Kyung Taec Kim | - |
dc.contributor.author | Hyung Taek Kim | - |
dc.contributor.author | Chang Hee Nam | - |
dc.date.available | 2015-09-01T01:19:56Z | - |
dc.date.created | 2015-05-18 | ko |
dc.date.issued | 2015-04 | - |
dc.identifier.issn | 0031-9007 | - |
dc.identifier.uri | https://pr.ibs.re.kr/handle/8788114/1770 | - |
dc.description.abstract | High-harmonic radiation emitted from molecules in a strong laser field contains information on molecular structure and dynamics. When multiple molecular orbitals participate in high-harmonic generation, resolving the contribution of each orbital is crucial for understanding molecular dynamics and for extending high-harmonic spectroscopy to more complicated molecules. We show that two-dimensional high-harmonic spectroscopy can resolve high-harmonic radiation emitted from the two highest-occupied molecular orbitals, HOMO and HOMO-1, of aligned molecules. By the application of an orthogonally polarized two-color laser field that consists of the fundamental and its second-harmonic fields to aligned CO2 molecules, the characteristics attributed to the two orbitals are found to be separately imprinted in odd and even harmonics. Two-dimensional high-harmonic spectroscopy may open a new route to investigate ultrafast molecular dynamics during chemical processes | - |
dc.description.uri | 1 | - |
dc.language | 영어 | - |
dc.publisher | AMER PHYSICAL SOC | - |
dc.title | Resolving Multiple Molecular Orbitals Using Two-Dimensional High-Harmonic Spectroscopy | - |
dc.type | Article | - |
dc.type.rims | ART | - |
dc.identifier.wosid | 000352788100004 | - |
dc.identifier.scopusid | 2-s2.0-84929601145 | - |
dc.identifier.rimsid | 19520 | ko |
dc.date.tcdate | 2018-10-01 | - |
dc.contributor.affiliatedAuthor | Hyeok Yun | - |
dc.contributor.affiliatedAuthor | Kyung-Min Lee | - |
dc.contributor.affiliatedAuthor | Jae Hee Sung | - |
dc.contributor.affiliatedAuthor | Kyung Taec Kim | - |
dc.contributor.affiliatedAuthor | Hyung Taek Kim | - |
dc.contributor.affiliatedAuthor | Chang Hee Nam | - |
dc.identifier.doi | 10.1103/PhysRevLett.114.153901 | - |
dc.identifier.bibliographicCitation | PHYSICAL REVIEW LETTERS, v.114, no.15, pp.153901 | - |
dc.citation.title | PHYSICAL REVIEW LETTERS | - |
dc.citation.volume | 114 | - |
dc.citation.number | 15 | - |
dc.citation.startPage | 153901 | - |
dc.date.scptcdate | 2018-10-01 | - |
dc.description.wostc | 13 | - |
dc.description.scptc | 15 | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordPlus | GENERATION | - |
dc.subject.keywordPlus | FIELD | - |
dc.subject.keywordPlus | PSEUDOPOTENTIALS | - |
dc.subject.keywordPlus | TIME | - |