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Jinwon, Jeon
분자활성 촉매반응 연구단
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Regio- and Stereoselective Functionalization Enabled by Bidentate Directing Groups

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Title
Regio- and Stereoselective Functionalization Enabled by Bidentate Directing Groups
Author(s)
Jinwon Jeon; Changseok Lee; Inyoung Park; Sungwoo Hong
Publication Date
2021-12
Journal
Chemical Record, v.21, no.12, pp.3613 - 3627
Publisher
John Wiley and Sons Inc
Abstract
© 2021 The Chemical Society of Japan & Wiley-VCH GmbHChelation-assisted C−H bond and alkene functionalization using bidentate directing groups offers an elegant and versatile approach to overcome regiocontrol issues by allowing the catalyst to come into close proximity with the targeted sites. In this personal account, we highlight our recent works in developing regio- and stereocontrolled functionalizations through transition-metal catalysis enabled by bidentate directing groups. We classify our results into two categories: (1) regioselective alkene functionalization using bidentate directing groups, and (2) asymmetric C–H functionalization using chiral bidentate directing groups. Furthermore, density functional theory studies to elucidate the origin of the regio- and stereoselectivity exerted by bidentate directing groups are discussed.
URI
https://pr.ibs.re.kr/handle/8788114/11010
DOI
10.1002/tcr.202100117
ISSN
1527-8999
Appears in Collections:
Center for Catalytic Hydrocarbon Functionalizations(분자활성 촉매반응 연구단) > 1. Journal Papers (저널논문)
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