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Synthesis and Photophysical Properties of Hexabenzocoronene-Tetrabenzoporphyrin Architectures

DC Field Value Language
dc.contributor.authorMichael Ruppel-
dc.contributor.authorLampros‐Pascal Gazetas-
dc.contributor.authorDominik Lungerich-
dc.contributor.authorNorbert Jux-
dc.date.accessioned2021-01-11T00:50:00Z-
dc.date.accessioned2021-01-11T00:50:00Z-
dc.date.available2021-01-11T00:50:00Z-
dc.date.available2021-01-11T00:50:00Z-
dc.date.created2020-10-16-
dc.date.issued2020-10-
dc.identifier.issn1434-193X-
dc.identifier.urihttps://pr.ibs.re.kr/handle/8788114/9020-
dc.description.abstractPorphyrin-based architectures have emerged as excellent candidates for artificial light-harvesting antennae. Although tetrabenzoporphyrins (TBPs), the pi-extended "bigger brothers" of porphyrins, benefit from increased absorptivity in the near-infrared (NIR), their utilization in light-harvesting systems is still in its infancy. Within this work, we prepared two donor-acceptor hetero dyads consisting of hexa-peri-hexabenzocoronenes (HBCs) to harvest high energetic near-UV light, and a TBP core, which serves as visible to NIR light antenna and as subsequent energy sink of the conjugate. The HBCs are either attached to themeso-position or via a maleimide-bridge on the periphery of the macrocycle. Upon excitation of the HBC moieties, both dyads exhibit an efficient energy transfer to the TBP core. Furthermore, the TBP-HBC dyads show superior light-harvesting properties compared to the respective HBC-porphyrin reference and the naturally occurring chlorophylls a/b-
dc.description.uri1-
dc.language영어-
dc.publisherJohn Wiley & Sons Ltd.-
dc.titleSynthesis and Photophysical Properties of Hexabenzocoronene-Tetrabenzoporphyrin Architectures-
dc.typeArticle-
dc.type.rimsART-
dc.identifier.wosid000563895600001-
dc.identifier.scopusid2-s2.0-85089700646-
dc.identifier.rimsid73070-
dc.contributor.affiliatedAuthorDominik Lungerich-
dc.identifier.doi10.1002/ejoc.202000860-
dc.identifier.bibliographicCitationEuropean Journal of Organic Chemistry, v.2020, no.40, pp.6352 - 6360-
dc.citation.titleEuropean Journal of Organic Chemistry-
dc.citation.volume2020-
dc.citation.number40-
dc.citation.startPage6352-
dc.citation.endPage6360-
dc.description.journalClass1-
dc.description.isOpenAccessN-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.subject.keywordPlusPORPHYRIN-ZINC PHTHALOCYANINE-
dc.subject.keywordPlusEXCITATION-ENERGY TRANSFER-
dc.subject.keywordPlusARTIFICIAL PHOTOSYNTHESIS-
dc.subject.keywordPlusMULTIPORPHYRIN ARRAYS-
dc.subject.keywordPlusPHOTOINDUCED ENERGY-
dc.subject.keywordPlusQUANTUM DOTS-
dc.subject.keywordPlusEFFICIENT-
dc.subject.keywordPlusELECTRON-
dc.subject.keywordPlusSINGLET-
dc.subject.keywordPlusPERYLENE-
dc.subject.keywordAuthorCoronenes-
dc.subject.keywordAuthorDonor-acceptor systems-
dc.subject.keywordAuthorExcited energy transfer-
dc.subject.keywordAuthorPorphyrins-
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Center for Nanomedicine (나노의학 연구단) > 1. Journal Papers (저널논문)
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